石墨相氮化碳光催化抗菌優(yōu)化策略及應(yīng)用研究進(jìn)展

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中圖分類號(hào):0643.36;0644.1 文獻(xiàn)標(biāo)識(shí)碼:A DOI:10.7535/hbkd.2025yx03005
Research progress on optimization strategies and applications of photocatalytic antibacterial activity of graphitic carbon nitride
I Wenhui1,WANG Ruopeng1,HAN Yuhe1,WANG Sai1, ZHANG Yumei12,LU Qiong 1,2 ,AN Jing 1,2
(1.School of Sciences,Hebei Universityof Science and Technology,Shijiazhuang,Hebei O50o18,China; .Hebei Provincial KeyLaboratoryof Photoelectric Controlon Surfaceand Interface,Shijiazhuang,Hebei O5oo18,China)
Abstract: Graphitic carbon nitride (g-C3N4 ) is a carbon-based conjugated polymer material with a crystal structure similar to graphite,which exhibitsunique potential inthe fieldof photocatalyticantibacterial activity.However,factorssuch as easy recombination of photogenerated electron Ξ(e-) -hole (h+ )pairs,incomplete sunlight absorption,small specific surface area, and poor adsorption propertiesof g-C3N4 photocatalysts leaded to low photocatalytic eficiency,limiting their antibacterial efectiveess.Toovercome theseproblems,strategies suchas morphologycontrol,precious metaldeposition,elementdoping, and heterostructure construction were employed to functionalize g-C3N4 and fully activated its antibacterial potential. A detailed introduction was given to the optimization strategies for the photocatalytic antibacterial performance of g-C3N4 ,with a focus on thecurrent stateofresearchonitsphotocatalyticantibacterial propertiesin waterdisinfection,antibacterial dresings, antibacterial textiles,and food packaging.The challenges currently faced in the development of g-C3N4 photocatalytic antibacterialagentswerehighlighted.Inordertoaddresstheinreasinglyseverechalengeofmicrobialcontamination,future research directions are suggested:1) depening the research onthe mechanisms of reactive oxygen species(ROS) induced damage to bacterialcellmembranes,intracellular proteins,DNA,etal;2)exploring the antibacterialapplications of g-C3N4 on broad-spectrum bacteria such as drug-resistant bacteria and commonly used fungi; 3) enhancing the adaptability of g-C3N4 in different environments.
Keywords:catalytic chemistry;graphitic carbon nitride;photocatalysis;antibacterial;optimization strategy
受環(huán)境變化和人類活動(dòng)的影響,病原體的傳播風(fēng)險(xiǎn)增加,公眾在飲用水、使用公共設(shè)施以及處理傷口時(shí),很容易感染具有傳染性和致病性的微生物。(剩余23910字)